长江中下游典型沿江城市内湖沉积物氮磷及有机质分布特征识别与溯源解析
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1.河海大学环境学院,浅水湖泊综合治理与资源开发教育部重点实验室,南京 210098 ;2.江苏省南京市江宁区水务局,南京 211100 ;3.河海大学设计研究院有限公司,南京 210098

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国家重点研发计划项目(2023YFC3208904,2023YFC3208900)资助


Identification and traceability analysis of the distribution characteristics of nitrogen, phosphorus and organic matter in inner lake sediments of typical riverine cities in the middle and lower reaches of the Yangtze River
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1.Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, Nanjing 210098 , P.R.China ;2.Nanjing Jiangning District Water Affairs Bureau, Jiangsu Province, Nanjing 211100 , P.R.China ;3.Hohai University Design & Research Institute Co., Ltd, Nanjing 210098 , P.R.China

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    摘要:

    湖泊沉积物参与水体元素循环重要环节,是目前水体富营养化的治理难点之一。为揭示城市内湖沉积物总氮(TN)、总磷(TP)和有机质(OM)污染特征及来源,并为水环境综合治理的环境效应评估提供新溯源视角,采集并测定了长江中下游典型沿江城市黄冈市遗爱湖25个点位沉积物柱状样中的TN、TP和OM含量,监测湖泊9个点位与排口溢流污水水质,解析湖泊水质与沉积物N、P和OM的空间分布特征,采用综合污染指数法定量评估沉积物TN、TP和OM污染风险,利用聚类分析和化学计量特征相结合的手段对湖泊沉积物N、P和OM来源进行定性识别和定量解析。结果表明:水平分布上,沉积物TN、TP和OM含量范围分别为940~3677 mg/kg、323~1667 mg/kg和1.03%~7.44%,空间分布差异大,且TN、TP和OM高值区集中在湖泊沿岸及排口附近。垂向上总体表现为表层>中、底层,表层沉积物中TN、TP和OM含量范围分别为920~4450 mg/kg、208~1970 mg/kg和2.05%~7.48%,表层TP含量高于中国东部浅水湖泊平均值,与国内沉积物污染严重的湖泊水平相近。综合污染指数法显示,表层沉积物TP污染严重,76%的湖区TP处于中度及重度污染状态,TN污染和综合污染程度较低。聚类分析-化学计量特征结果表明,溢流污染累积处沉积物C/N为11,遗爱湖表层沉积物C/N值为10.67,C/P值在20.16~190.97之间,约44%的OM来自藻类死亡后的分解释放,同时受20%溢流排放和36%面源污染的共同影响,TP主要来自面源污染,其次为溢流污水,TN的来源与OM相似。

    Abstract:

    Lake sediments play a crucial role in the elemental cycling of water bodies and represent one of the current challenges in managing eutrophication. To uncover the pollution characteristics and sources of total nitrogen (TN), total phosphorus (TP), and organic matter (OM) in the sediments of urban lakes and provide a new traceability perspective for assessing the environmental effects of comprehensive water environment management, this study collected and measured TN, TP, and OM contents in sediment points from 25 sites in Lake Yiai, Huanggang City. Water quality at nine lake sampling sites and at CSO (combined sewer overflow) outlet was monitored. Analyze the spatial distribution characteristics of TN, TP, and OM in lake water and sediment. The comprehensive pollution index method was employed to quantitatively assess the pollution risks of TN, TP, and OM in the sediments. Cluster analysis combined with stoichiometric characteristics was used to qualitatively identify and quantitatively analyze the sources of N, P, and OM in lake sediments. The results indicate that: There were spatial differences in the distribution of TN, TP and OM in sediments. The horizontal distribution of TN, TP and OM contents ranged from 940-3677 mg/kg, 323-1667 mg/kg and 1.03%-7.44%, the high-concentration sites of TN, TP, and OM were concentrated along the lake shores and near the discharge outlets. Vertically, the overall trend showed that the surface layer had higher concentrations than the middle and bottom layers. Specifically, the content ranges of TN, TP, and OM in the surface sediments were 920-4450 mg/kg, 208-1970 mg/kg and 2.05%-7.48%, respectively. The TP content of surface sediments was higher than the average value of shallow lakes in eastern China, and was similar to the level of lakes with serious sediment pollution in China. The comprehensive pollution index method revealed severe TP pollution in the surface sediments, with 76% of the lake area experiencing moderate to severe TP pollution, while TN pollution and overall pollution levels were relatively low. Cluster analysis combined with stoichiometric characteristics showed that the C/N ratio in sediments at locations with CSO pollution was 11, and the C/N ratio in the surface sediments of Lake Yiai was 10.67, with C/P values ranging from 20.16 to 190.97. Approximately 44% of OM originated from the decomposition of dead algae, while 20% was influenced by overflow discharges and 36% by diffuse pollution. TP primarily came from diffuse pollution, followed by overflow sewage, while the sources of TN were similar to those of OM.

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杨紫瑄,陈庠,李一平,王煜,朱晓琳,鲍航通,潘泓哲,章双双,严春敏.长江中下游典型沿江城市内湖沉积物氮磷及有机质分布特征识别与溯源解析.湖泊科学,2025,37(5):1523-1536. Yang Zixuan, Chen Xiang, Li Yiping, Wang Yu, Zhu Xiaolin, Bao Hangtong, Pan Hongzhe, Zhang Shuangshuang, Yan Chunmin. Identification and traceability analysis of the distribution characteristics of nitrogen, phosphorus and organic matter in inner lake sediments of typical riverine cities in the middle and lower reaches of the Yangtze River. Journal of Lake Sciences,2025,37(5):1523-1536. DOI:10.18307/2025.0513

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  • 收稿日期:2024-11-05
  • 最后修改日期:2025-01-13
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  • 在线发布日期: 2025-09-07
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